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class="ss"><div><span>导读： </span>激子是半导体中最基本的准粒子之一，是发展高效率光电器件和量子技术的核心。在传统三维半导体中，激子束缚能通常较弱，极大地限制了其在室温激子器件及量子科技应用中的发展。β-ZnTe(en)0.5是一种长程有序且稳定的 ...</div> </div> <!--[diy=diysummarybottom]--><div id="diysummarybottom" class="area"></div><!--[/diy]--> <div class="d"> <!--[diy=diycontenttop]--><div id="diycontenttop" class="area"></div><!--[/diy]--> <table cellpadding="0" cellspacing="0" class="vwtb"><tr><td id="article_content"><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; font-family: 微软雅黑; color: rgb(68, 68, 68); background-color: rgb(255, 255, 255); text-indent: 2em; text-align: justify; margin-bottom: 26px !important; line-height: 32px !important;">激子是<a href="http://sensor.oecr.com" target="_blank" class="relatedlink">半导体</a>中最基本的准粒子之一，是发展高效率光电器件和量子技术的核心。在传统三维半导体中，激子束缚能通常较弱，极大地限制了其在室温激子器件及量子科技应用中的发展。β-ZnTe(en)<sub style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; font-size: 16px !important; line-height: 32px !important;">0.5</sub>是一种长程有序且稳定的三维有机—无机杂化半导体，该<a href="http://material.oecr.com" target="_blank" class="relatedlink">材料</a>可能具有巨大的激子束缚能。</p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; font-family: 微软雅黑; color: rgb(68, 68, 68); background-color: rgb(255, 255, 255); text-indent: 2em; text-align: justify; margin-bottom: 26px !important; line-height: 32px !important;">最近，中国科学院半导体研究所研究员谭平恒团队与合作者，利用一种结合单光子荧光与双光子荧光激<a href="http://light.oecr.com" target="_blank" class="relatedlink">发光</a>谱的联合<a href="http://opticaltest.oecr.com" target="_blank" class="relatedlink">测量</a>方法，成功估算了β-ZnTe(en)<sub style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; font-size: 16px !important; line-height: 32px !important;">0.5</sub>的激子束缚能。该方法利用了单光子跃迁与双光子跃迁遵循不同选择定则的特性：单光子过程只能探测具有偶宇称的激子态（如1<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">s</em>基态），而双光子过程则可以探测具有奇宇称的激子态（如2<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">p</em>激发态）。通过精确测量1<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">s</em>态与2<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">p</em>态之间的能量差，并基于二维类氢模型进行分析，即可估算所测半导体材料的激子束缚能下限。</p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; font-family: 微软雅黑; color: rgb(68, 68, 68); background-color: rgb(255, 255, 255); text-indent: 2em; text-align: justify; margin-bottom: 26px !important; line-height: 32px !important;">研究团队依托自主设计研发的共聚焦显微拉曼模块，在室温下清晰地观测到了β-ZnTe(en)<sub style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; font-size: 16px !important; line-height: 32px !important;">0.5</sub>样品位于3.56eV的激子基态（1<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">s</em>）发光，并在双光子激发谱中发现了对应于激子激发态（2<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">p</em>）的共振吸收峰，二者能量差高达280meV。基于此，计算得出的激子束缚能超过315meV。该值是传统体相ZnTe半导体（约13meV）的二十余倍，也是目前已报道的三维半导体材料中的最高值，甚至可与典型的二维半导体相媲美。</p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; font-family: 微软雅黑; color: rgb(68, 68, 68); background-color: rgb(255, 255, 255); text-indent: 2em; text-align: justify; margin-bottom: 26px !important; line-height: 32px !important;">该三维杂化材料中巨大的激子束缚能，源于其独特的“三维框架、二维内核”的超晶格结构。其中，有机分子层不仅作为无机ZnTe片层之间的间隔物，构建了稳固的三维结构，更充当了<a href="http://electronic.oecr.com" target="_blank" class="relatedlink">电子</a>限域的势垒和介电屏蔽的调制层，从而极大地增强了电子与空穴之间的库仑相互作用，赋予了该三维材料类似二维材料的强激子效应。</p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; font-family: 微软雅黑; color: rgb(68, 68, 68); background-color: rgb(255, 255, 255); text-indent: 2em; text-align: justify; margin-bottom: 26px !important; line-height: 32px !important;">相关研究成果发表在《美国化学会志》（<em style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; margin-bottom: 26px !important; line-height: 32px !important;">Journal of the American Chemical Society</em>）上。</p><p style="text-align: center;"><a href="data/attachment/portal/202511/12/100131uwpmr6z3p2pomj22.png" target="_blank"><img src="data/attachment/portal/202511/12/100131uwpmr6z3p2pomj22.png"></a></p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; line-height: 1.5em; font-family: 微软雅黑; color: rgb(68, 68, 68); text-indent: 0em; background-color: rgb(255, 255, 255); text-align: center; margin-bottom: 26px !important;"><span style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; line-height: 1.5em; margin-bottom: 26px !important;"></span>三维有机无机杂化半导体激子特性研究取得进展</p><p style="margin-top: 0px; margin-right: 0px; margin-left: 0px; padding: 0px; border: 0px; list-style: none; font-size: 16px; line-height: 1.5em; font-family: 微软雅黑; color: rgb(68, 68, 68); text-indent: 0em; background-color: rgb(255, 255, 255); text-align: center; margin-bottom: 26px !important;"><br></p><p microsoft="" yahei",="" simsun;="" 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